Based on NDR (ournmailserver.com #5.3.3 smtp;500 5.3.3 Unrecognized command) it looks your Exchange server is not able to communicate with remote email system.
1> have you observed any such issues with any other outgoing emails?
2> if no - this problem is with remote email system which you can only inform them and wait till it gets fixed.
3> if yes - you need to check what changes you have done in your exchange server recently.